Search results for "frequency dispersion"

showing 4 items of 4 documents

Non-linear optical, electrochemical and spectroelectrochemical properties of amphiphilic inner salt porphyrinic systems

2016

Three zwitterionic meso-substituted A3B- and AB2C-porphyrins containing one sulfonato alkylpyridinium substituent and three or two alkoxy-substituted phenyl groups were synthesized in good yield and fully characterized as to their physicochemical properties by a variety of techniques. This new series of inner salt donor-acceptor meso-substituted porphyrin derivatives were prepared for possible application as amphiphilic probes for membrane insertion in the area of combined second-harmonic and two-photon fluorescence cellular microscopy. To this end, the linear and nonlinear optical properties of the compounds were characterized, together with their electrochemical and spectroelectrochemica…

designInorganic chemistrySubstituentamphiphilic inner salt02 engineering and technology010402 general chemistryElectrochemistryPhotochemistry[ CHIM ] Chemical Scienceselectron-accepting moieties01 natural sciencesnon-linear optical propertychemistry.chemical_compoundAmphiphilechromophores[CHIM]Chemical SciencesMoleculeChemistryfrequency dispersionSecond-harmonic generationspectroelectrochemistrydipolar complexesGeneral Chemistry021001 nanoscience & nanotechnologyPorphyrinFluorescence0104 chemical sciences2nd-harmonic generationelectrochemistrymicroscopycharge-transferfluorescenceAbsorption (chemistry)hyper-rayleigh scattering0210 nano-technologyJournal of Porphyrins and Phthalocyanines
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Broadband Dielectric Spectroscopy of PSN-Rich PMN-PSN Ceramics

2008

The broadband dielectric permittivity of ordered 0.1PMN-0.9PSN and disordered 0.2PMN-0.8PSN ceramics was investigated. The anomaly of dielectric permittivity is clearly seen in the region of 370 K for 0.1 PMN-0.9 PSN at all frequencies. 0.2 PMN-0.8 PSN shows relaxor behaviour with huge frequency dispersion below 350 K. Calculated distribution of relaxation times shows noticeable influence of polar nano regions to the total dielectric spectrum below 320 K with the longest relaxation times edge diverging according to the Vogel-Fulcher law. In 0.1 PMN-0.9 PSN two a little overlapped peaks present in the distribution of relaxation times, influenced by displacive lead motions at high frequencies…

Materials scienceCondensed matter physicsConductivityCondensed Matter PhysicsElectronic Optical and Magnetic MaterialsNuclear magnetic resonancevisual_artFrequency dispersionNano-visual_art.visual_art_mediumRelaxation (physics)PolarCeramicAnomaly (physics)Broadband dielectric spectroscopyFerroelectrics
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Uniaxial Pressure Effects on the Dielectric Properties of the PLZT-x/65/35 (x = 9.75 and 10) Ceramics

2012

The influence of uniaxial pressure (0-1000 bars) applied parallel to the ac electric field on the dielectric properties of PLZT-x/65/35 ceramics (x = 9.75 and 10) was investigated. The results show that the applied stress has a significant influence on the dielectric properties of PLZT ceramics. Applying uniaxial pressure leads to the reduction of the electric permittivity (ϵ) peak and the frequency dispersion. Moreover, the peak of ϵ becomes diffuse and shifts to a higher temperature with increasing pressure. The results show that applying uniaxial pressure induces similar effects as the increase in Ti−ion concentration in the PZT system. We interpreted our results based on the domain swit…

PermittivityMaterials scienceDielectricCondensed Matter PhysicsUniaxial pressureFerroelectricityElectronic Optical and Magnetic MaterialsStress (mechanics)visual_artElectric fieldFrequency dispersionvisual_art.visual_art_mediumCeramicComposite materialFerroelectrics
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Influence of Uniaxial Pressure on Dielectric Properties of the PLZT-x/65/35 (x = 11 and 13) Ceramics

2012

Uniaxial pressure (0–1000 bars) effects on the dielectric properties of the PLZT-x/65/35 ceramic samples (x = 11 and 13) samples was investigated. The obtained results reveal that the applied stress largely changes the dielectric properties of these ceramics. Applying uniaxial pressure leads to a reduction of the peak intensity of the electric permittivity and a change of the frequency dispersion. Besides with increasing the pressure the ϵ-peak shifts to a higher temperature. The results show that applying the uniaxial pressure induces similar effects as increasing the Ti−ion concentration in PZT system. These effects can be connected with the change in domain structure under the action of …

Stress (mechanics)PermittivityMaterials scienceFrequency dispersionvisual_artPeak intensityvisual_art.visual_art_mediumCeramicDielectricComposite materialCondensed Matter PhysicsUniaxial pressureElectronic Optical and Magnetic MaterialsFerroelectrics
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